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We have synthesized Cu-substituted (Au,Cu) Al Yb quasicrystals in order to investigate the relationship between the quasilattice constant and the magnetic property. The quasilattice constant a R is found to decrease as Au is replaced by Cu, and the maximum reduction of 2.18% in aR was observed for x = 0.60 in (Au1-xCux)(49)Al34Yb17. Magnetic measurements of (Au1-xCux)(49)Al34Yb17 (x = 0, 0.10, 0.20, 0.50) show that the intermediate-valence state of Yb persists in all the studied compositions. The effective magnetic moment is found to depend on (r) over bar /a(R) rather than on the quasilattice constant a(R). This suggests that f/ari can be regarded as a measure of the chemical pressure induced on the Yb atoms.

Magnetic Properties of Icosahedral (Au,Cu)-Al-Yb Quasicrystals