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Based on crystal-and ligand-field theory, double-spin-orbital coupling approach was used to analyze the crystal-field energy levels and spin-Hamiltonian parameters of Ni2+ ion at trigonal site in CdBr2. The local lattice distortion (Delta R and tau(Ni24+)) is estimated from the crystal field parameters; the crystal field energy Hamiltonian was diagonalized in the full basis consisting of 45 wave functions of the Ni2+ ion. Results of calculations are in good agreement with experimental data. The reasonableness of the theoretical results is discussed.

Explanation of the Optical Spectra and Spin-Hamiltonian Parameters for Nickel(II) in Cadmium Bromide Crystal