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Resonant microwave radiation applied to a single crystal of the molecularmagnet Fe_8 induces dramatic changes in the sample's magnetization. Transitionsbetween excited states are found even though at the nominal system temperaturethese levels have negligible population. We find evidence that the sample heatssignificantly when the resonance condition is met. In addition, heating isobserved after a short pulse of intense radiation has been turned off,indicating that the spin system is out of equilibrium with the lattice.Comment: Version to appear in Europhysics Letters. Minor changes and updated  reference

Non-equilibrium magnetization dynamics in the Fe 8 single-molecule magnet induced by high-intensity microwave radiation

Non-equilibrium magnetization dynamics in the Fe ₈ single-molecule magnet induced by high-intensity microwave radiation