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In this supplementary material, we recollect, for reader's convenience, thegeneral scheme of suggested multiscale model (Sec. 1), and basic informationsabout approaches used for pilot study: a detailed description of theinteraction model (Sec. 2) and dynamical methods used for the dark dynamicsstep (Sec. 3) reported previously in two preceding studies [1, 2]. In addition,a detailed description of the treatment of radiative processes is also given(Sec. 4).

Multiscale non-adiabatic dynamics with radiative decay, case study on the post-ionization fragmentation of rare-gas tetramers