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Comprehensive experimental studies by magnetic, thermal and neutronmeasurements have clarified that Rb4Mn(MoO4)3 is a model system of a quasi-2Dtriangular Heisenberg antiferromagnet with an easy-axis anisotropy, exhibitingsuccessive transitions across an intermediate collinear phase. As a rare casefor geometrically frustrated magnetism, quantitative agreement betweenexperiment and theory is found for complete, anisotropic phase diagrams as wellas magnetic properties.

Successive phase transitions and phase diagrams of the quasi-two-dimensional triangular antiferromagnet Rb4Mn(MoO4)3