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We report a comparative study of the series Fe1.1Te1-xSex and thestoichiometric FeTe1-xSex to bring out the difference in their magnetic,superconducting and electronic properties. The Fe1.1Te1-xSex series is found tobe magnetic and its microscopic properties are elucidated through Moessbauerspectroscopy. The magnetic phase diagram of Fe1.1Te1-xSex is traced out and itshows the emergence of spin-glass state when the antiferromagnetic state isdestabilized by the Se substitution. The isomer shift and quadrupolar splittingobtained from the Moessbauer spectroscopy clearly brings out the electronicdifferences in these two series.

Magnetic phase diagram of Fe1.1Te1-xSex: A comparative study with the stoichiometric superconducting FeTe1-xSex system