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Molecular dynamics simulations for aqueous sodium chloride solutions werecarried out at various concentrations. Supplementary to the Debye-H\"uckeltheory, reversible transient nucleation of ions was observed even in dilutesolutions. The average size of formed ion clusters and the lifetime of ionpairs increase with concentration until the saturation point, when ion clustersbecome stable and individual ions adjust their positions to form orderedlattice structures, leading to irreversible ion crystallization, which isbeyond the description of the classical nucleation theory.

Reversible Transient Nucleation in Ionic Solutions as the Precursor of Ion Crystallization