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Thermal and photo responsive copolymer based on  N -vinylamide backbone was designed. Methoxyethyl group and azobenzene were selected to improve hydrophilicity and photoresponsive moieties, respectively. The  N -(methoxyethyl)- N -vinylformamide was synthesized and copolymerized with  N -vinylformamide by free radical polymerization. In order to control the nanosized structures, poly( N -vinylformamide) derivatives bearing azobenzene at the  N -position near to the vinyl polymer main chain were synthesized by polymer reaction with the poly( N -vinylformamide- co - N -(methoxyethyl)- N -vinylformamide) and azobenzene. Aggregation size of the multi-stimuli-responsive polymer was controlled by preparation of the hydrophobic interaction at around  N -position.   Electronic supplementary material  The online version of this article (doi:10.1186/s11671-017-2221-7) contains supplementary material, which is available to authorized users.

Aggregation Control by Multi-stimuli-Responsive Poly(N-vinylamide) Derivatives in Aqueous System