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Optical and FTIR spectroscopy was employed to study the properties of 80GeS 2 -20Ga 2 S 3 -CsCl chalcohalide glasses with CsCl additives in a temperature range of 77–293 K. It is shown that CsCl content results in the shift of fundamental absorption edge in the visible region. Vibrational bands in FTIR spectra of (80GeS 2 -20Ga 2 S 3 ) 100 −  х  (СsCl)  x   ( x  = 5, 10, and 15) are identified near 2500 cm −1 , 3700 cm −1 , ,  around 1580 cm −1 , and a feature at 1100 cm −1 . Low energy shifts of vibrational frequencies in glasses with a higher amount of CsCl can be caused by possible thermal expansion of the lattice and nanovoid agglomeration formed by CsCl additives in the inner structure of the Ge-Ga-S glass.

Optical and Vibrational Spectra of CsCl-Enriched GeS2-Ga2S3 Glasses