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A new composite system, Ba(Zr 0.07 Ti 0.93 )O 3  (BZT93) ceramic/NiO nanoparticles, was fabricated to investigate the effect of NiO nanoparticles on the properties of these composites.  M-H  hysteresis loops showed an improvement in the magnetic behavior for higher NiO content samples plus modified ferroelectric properties. However, the 1 vol.% samples showed the optimum ferroelectric and ferromagnetic properties. Examination of the dielectric spectra showed that the NiO additive promoted a diffuse phase transition, and the two phase transition temperatures, as observed for BZT93, merged into a single phase transition temperature for the composite samples.

Effects of NiO nanoparticles on the magnetic properties and diffuse phase transition of BZT/NiO composites