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A novel photochromic compound with NH-N intramolecular H-bond (1-p-toluenesulphonylazo-2,4,6,8-tetrakis(tert-butyl)phenoxazine) and the corresponding model structures (1-oxo-2,4,6,8-tetrakis(tertbutyl)phenoxazine, 2,4,5,7-tetrakis (tert-butyl )-1-( veratroylazo ) phenoxazine, 2,4,5,7-tetrakis ( tert-butyl )-Nacetyl-1-(p-toluenesulphonylazo)phenoxazine) have been synthesized and their spectral and photochemicalproperties are studied. The photochromic transformations observed are found to be conditioned by ESIPT(as a primary step) followed by E-Z isomerisation about N–N-bond

Photoinitiated azo-hydrazo tautomerizm of 1-p- toluenesulphonylazo-2,4,6,8-tetrakis (tert-butyl)phenoxazine