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Ag+/ZSM-5 catalysts were prepared by an ion-exchange method. UV-irradiation of the Ag+/ZSM-5 catalysts in the presence of N2O led to the photocatalytic decomposition of N2O into N2 and O2 at 298 K. Investigations of the effective wavelength of the irradiated UV-light for the reaction as well as the in-situcharacterization of the catalysts by means of UV-Vis, photoluminescence and FT-IR spectroscopies revealedthat the photoexcitation of the Ag+ − N2O complexes formed between gaseous N2O and the isolated Ag+ ions exchanged within the zeolite cavities plays a significant role in the reaction

international journal of photoenergy

Incorporation of silver (I) ions within zeolite cavities and their photocatalytic reactivity for the decomposition of<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" alttext="${\text{N}}_{\text{2}} {\text{O}}$"><mml:mrow><mml:msub><mml:mtext>N</mml:mtext><mml:mtext>2</mml:mtext></mml:msub><mml:mtext>O</mml:mtext></mml:mrow></mml:math>into<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" alttext="${\text{N}}_{\text{2}} $"><mml:mrow><mml:msub><mml:mtext>N</mml:mtext><mml:mtext>2</…

Incorporation of silver (I) ions within zeolite cavities and their photocatalytic reactivity for the decomposition ofN2OintoN2