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We investigated a promising three-step resonance ionization scheme of strontium (Sr) 5s 2  1 S 0  ⟶ 5s5p  3P    1    ° ⟶ 5s5d  3 D 2  ⟶ 4dnp (or 4dnf,  n  = 39) using the first-step intercombination transition for the enhancement of isotope selectivity. The power broadening observed in the 2 nd  transition indicates that laser power of less than 0.2 mW is sufficient for saturating this transition. Isotope separation can be successfully expected with application of the 3 rd  transition due to the narrow width of the 4dnp (or 4dnf,  n  = 39) autoionization level, paving the way for analysis of trace  90 Sr in environmental applications.

journal of spectroscopy

Investigation of Optical Ionization of Strontium via 5s21S0 ⟶ 5s5p 3<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" id="M1"><mml:mrow><mml:msubsup><mml:mrow><mml:mtext>P</mml:mtext></mml:mrow><mml:mrow><mml:mn mathvariant="bold">1</mml:mn></mml:mrow><mml:mrow><mml:mo>°</mml:mo></mml:mrow></mml:msubsup></mml:mrow></mml:math> ⟶ 5s5d 3D2 ⟶ 4dnp (or 4ndf, n = 39) for Isotope Selectivity Enhancement

Investigation of Optical Ionization of Strontium via 5s21S0 ⟶ 5s5p 3P1° ⟶ 5s5d 3D2 ⟶ 4dnp (or 4ndf, n = 39) for Isotope Selectivity Enhancement

Investigation of Optical Ionization of Strontium via 5s²¹S₀ ⟶ 5s5p ³P1° ⟶ 5s5d ³D₂ ⟶ 4dnp (or 4ndf, n = 39) for Isotope Selectivity Enhancement