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We present charge transfer absorption, resonance Raman and time-resolved infrared spectral data for (CN)5FeCNRu(NH3)5− in various solvents. The transient infrared spectra and anisotropies reveal both non-equilibrium vibrational populations of high frequency modes and local solvent heating.

laser chemistry

Vibrational Mode Coupling to Reverse Electron Transfer in (CN)<sub>5</sub>FeCNRu<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msubsup><mml:mrow><mml:mrow><mml:mo>(</mml:mo><mml:mrow><mml:msub><mml:mrow><mml:mtext>NH</mml:mtext></mml:mrow><mml:mtext>3</mml:mtext></mml:msub></mml:mrow><mml:mo>)</mml:mo></mml:mrow></mml:mrow><mml:mn>5</mml:mn><mml:mo>−</mml:mo></mml:msubsup></mml:mrow></mml:math> in Solution

Vibrational Mode Coupling to Reverse Electron Transfer in (CN)5FeCNRu(NH3)5− in Solution

Vibrational Mode Coupling to Reverse Electron Transfer in (CN)₅FeCNRu(NH3)5− in Solution