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A homemade TEA CO 2  laser tuned to the 1OP(48) line, 10.91 μm, was used to excite thev  4     mode of CDCl 3  (914 cm -1 ). The IR fluorescence signal from the CDCl 3    2   v  5     overtone band (1492 cm -1 ) was isolated by means of a gaseous filter. The temporal variation of this fluorescence emission was studied as a function of the laser fluence. Under high excitation conditions, non-linear effects become obvious, and measured rate constants greater than predicted from linear kinetic rate equations have been found.

laser chemistry

Vibrational Relaxation of the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mn>2</mml:mn><mml:msub><mml:mi>v</mml:mi><mml:mn>5</mml:mn></mml:msub></mml:mrow></mml:math> Overtone of CDCl<sub>3</sub> Highly Excited by a Tea CO<sub>2</sub> Laser

Vibrational Relaxation of the 2v5 Overtone of CDCl3 Highly Excited by a Tea CO2 Laser

Vibrational Relaxation of the 2v5 Overtone of CDCl₃ Highly Excited by a Tea CO₂ Laser