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Golden SmS is a paramagnetic, mixed-valence system with a pseudogap. Withincreasing pressure across a critical pressure Pc, the system undergoes adiscontinuous transition into a metallic, anti-ferromagnetically ordered state.By using a combination of thermodynamic, transport, and magnetic measurements,we show that the pseudogap results from the formation of a local bound statewith spin singlet. We further argue that the transition Pc is regarded as atransition from an insulating electron-hole gas to a Kondo metal, i.e., from aspatially bound state to a Kondo virtually bound state between 4f andconduction electrons.

Discontinuous Transition from a Real Bound State to Virtual Bound State in a Mixed-Valence State of SmS