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Ultrafast wavepacket dynamics of electron-phonon-photon systems is studied bynumerical calculations. When nonadiabaticity of electron-phonon systems istaken into account, Raman scattering process plays an important role in thedynamics of the system. We found that the interplay of the electron-phononnonadiabaticity and the Raman scattering determines the wavepacket motionparticularly in the vicinity of the conical intersection of adiabatic potentialenergy surfaces, which shows that we should consider this effect in order toreveal the photoexcitation/deexcitation process of materials in femtosecondtime scale.

the european physical journal. d, atomic, molecular and optical physics/the european physical journal. d, atomic, molecular, optical and plasma physics

Interplay of electron-phonon nonadiabaticity and Raman scattering in the wavepacket dynamics of electron-phonon-photon systems