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We investigate the rovibrational population redistribution of polar moleculesin the electronic ground state induced by spontaneous emission and blackbodyradiation. As a model system we use optically trapped LiCs molecules formed byphotoassociation in an ultracold two-species gas. The population dynamics ofvibrational and rotational states is modeled using an ab-initio electric dipolemoment function and experimental potential energy curves. Comparison with theevolution of the v"=3 electronic ground state yields good qualitativeagreement. The analysis provides important input to assess applications ofultracold LiCs molecules in quantum simulation and ultracold chemistry.

the european physical journal. d, atomic, molecular and optical physics/the european physical journal. d, atomic, molecular, optical and plasma physics

Population redistribution in optically trapped polar molecules