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Understanding spin-lattice coupling represents a key challenge in moderncondensed matter physics, with crucial importance and implications forultrafast and 2D-magnetism. The efficiency of angular momentum and energytransfer between spins and the lattice imposes fundamental speed limits on theability to control spins in spintronics, magnonics and magnetic data storage.We report on an efficient nonlinear mechanism of spin-lattice coupling drivenby THz light pulses. A nearly single-cycle THz pulse resonantly interacts witha coherent magnonic state in the antiferromagnet CoF2 and excites theRaman-active THz phonon. The results reveal the unique functionality ofantiferromagnets allowing ultrafast spin-lattice coupling using light.

Terahertz-Light Driven Coupling of Antiferromagnetic Spins to Lattice