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We observe that when an ultracold ground state cesium (Cs) atom becomes boundwithin the electronic cloud of an extended Cs electronic orbit, ultralong-rangemolecules with giant (kilo-Debye) permanent electric dipole moments form. Largemolecular permanent electric dipole moments are challenging to experimentallyrealize. Meeting this challenge has garnered significant interest becausepermanent electric dipole moments are important for understanding symmetrybreaking in molecular physics, control of chemical reactions and realization ofstrongly correlated many-body quantum systems. These new hybrid class of`trilobite' molecules are predominated with degenerate Rydberg manifolds,making them difficult to produce with conventional optical association. Theirbehavior is quantitatively reproduced with detailed coupled-channelcalculations.

Production of trilobite Rydberg molecule dimers with thousand-Debye permanent electric dipole moments