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Atomic-level structural changes in materials are important but challenging tostudy. Here, we demonstrate the dynamics and the possibility of manipulating aphosphorus dopant atom in graphene using scanning transmission electronmicroscopy (STEM). The mechanisms of various processes are explored andcompared with those of other dopant species by first-principles calculations.This work paves the way for designing a more precise and optimized protocol foratomic engineering.

Competing dynamics of single phosphorus dopant in graphene with electron irradiation