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Laser cooling by collisional redistribution of radiation has beensuccessfully applied in the past for cooling dense atomic gases. Here we reporton progress of work aiming at the demonstration of redistribution laser coolingin a molecular gas. The candidate molecule strontium monohydride is produced bylaser ablation of strontium dihydride in a pressurized noble gas atmosphere.The composition of the ablation plasma plume is analyzed by measuring itsemission spectrum. The dynamics of SrH molecular density following the ablationlaser pulse is studied as a function of the buffer gas pressure and the laserintensity.

Towards redistribution laser cooling of molecular gases: Production of candidate molecules SrH by laser ablation