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The crystal structure of the anionic zinc–[amino(iminio)methyl]phosphonate one-dimensional coordination polymer, Zn-AIMP, is reported; the negative charge is balanced by an oxidanium cation (H 3 O + ) to give the composition {(H 3 O)[Zn(CH 4 N 2 PO 3 ) 3 ]} n . The building unit of the coordination polymer comprises a divalent Zn 2+  cation (site symmetry \overline3..) and three [amino(iminio)methyl]phosphonate mono-anionic ligands (point group symmetry  m ). The AIMP ligand exists in a zwitterionic form with a total charge −1 as the phosphonate is fully deprotonated (–PO 3 2− ), while the amino(iminio)methyl moiety is protonated (H 2 N—C—NH 2 + ).

catena-Poly[oxidanium [tris{μ-[amino(iminio)methyl]phosphonato}zincate(II)]]