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In the title compound, C 13 H 15 N 5 O 2 S, the acetamide N—C(=O)—C plane makes dihedral angles of 30.51 (11) and 51.93 (11)°, respectively, with the benzene ring and the pyrimidine ring. The dihedral angle between the benzene and pyrimidine rings is 43.40 (6)°. There is an intramolecular N—H...N hydrogen bond with an  S (7) ring motif. In the crystal, molecules are linked by pairs of intermolecular N—H...N hydrogen bonds, forming inversion dimers with an  R 2 2 (8) ring motif. The molecules are further linked by intermolecular N—H...O hydrogen bonds, forming a  C (9) chain along [100]. Intermolecular C—H...π and N—H...π interactions are also observed.

2-[(4,6-Diaminopyrimidin-2-yl)sulfanyl]-N-(4-methoxyphenyl)acetamide