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In the title salt, (C 16 H 36 N) 2 [Ni(C 6 N 4 S 2 ) 2 ], the centrosymmetric complex dianion is planar, with an r.m.s. deviation of 0.031 (1) Å. The Ni II  atom, lying on an inversion centre, has an almost undistorted square-planar coordination geometry, with Ni—S bond lengths of 2.1606 (5) and 2.1759 (5) Å.

Bis(tetra-n-butylammonium) bis(5,6-dicyanopyrazine-2,3-dithiolato-κ2 S,S′)nickelate(II)

Bis(tetra-n-butylammonium) bis(5,6-dicyanopyrazine-2,3-dithiolato-κ² S,S′)nickelate(II)