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The search for new mol-ecular materials with inter-esting magnetic properties using the pseudohalide azide ion and quinolin-8-amine (aqin, C 9 H 8 N 2 ) as a chelating ligand, led to the synthesis and structure determination of the title complex, [Fe(N 3 ) 2 (C 9 H 8 N 2 ) 2 ]. The complex shows an octa-hedral geometry, with the Fe II atom surrounded by six N atoms; the two N 3  - anions coordinate in a cis configuration, while the remaining N atoms originate from the two quinolin-8-amine ligands with the quinoline N atoms lying on opposite sides of the Fe atom. The crystal packing is dominated by layers of hydro-philic and aromatic regions parallel to the ac plane, stabilized by a two-dimensional hydrogen-bonded network and π-π stacking.

Crystal structure of bis(azido-κN)bis(quinolin-8-amine-κ2N,N′)iron(II)

Crystal structure of bis(azido-κN)bis(quinolin-8-amine-κ²N,N′)iron(II)