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In the title one-dimensional coordination polymer, [Mn(NCS) 3 (C 10 H 16 N 3 )]  n  , the Mn II  atom is coordinated by an  N , N ′-bidentate Schiff base and four thio­cyanate ligands in a distorted octa­hedral N 5 S geometry. Bridging thio­cyanate ligands inter­connect adjacent [Mn(NCS) 2 (C 10 H 16 N 3 )] units, giving rise to helical chains extending along the  b  axis. The chains are further linked through N—H⋯S hydrogen bonds, leading to a three-dimensional supra­molecular network.

catena-Poly[[(2-{[2-(dimethylammonio)ethyl]iminomethyl}pyridine-κ2N,N′)bis(thiocyanato-κN)manganese(II)]-μ-thiocyanato-κ2N:S]