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In the title compound, {[Nd(C 14 H 9 N 2 O 5 )(C 14 H 8 N 2 O 5 )]·2H 2 O}  n  , the Nd III  atom is eight-coordinated as it is surrounded by eight carboxyl­ate O atoms from six ligands in a distorted square-anti­prismatic arrangement. The Nd III  atoms are linked by H L−  and  L2−  ligands [H 2L  is 5-(pyridine-4-carboxamido)­isophthalic acid], forming a bilayer network. The layers are linked into a three-demensional network through N—H⋯O and O—H⋯O hydrogen bonds.

acta crystallographica. section e

Poly[[[μ<sub>3</sub>-5-(pyridine-4-carboxamido)isophthalato]{μ<sub>3</sub>-5-[(pyridin-1-ium-4-yl)carbonylamino]isophthalato}neodymium(III)] dihydrate]

Poly[[[μ3-5-(pyridine-4-carboxamido)isophthalato]{μ3-5-[(pyridin-1-ium-4-yl)carbonylamino]isophthalato}neodymium(III)] dihydrate]

Poly[[[μ₃-5-(pyridine-4-carboxamido)isophthalato]{μ₃-5-[(pyridin-1-ium-4-yl)carbonylamino]isophthalato}neodymium(III)] dihydrate]