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The title compound, (C 16 H 36 N) 3 [Th(NCS) 4 (NO 3 ) 3 ], was obtained from the reaction of Th(NO 3 ) 4 ·5H 2 O with (Bu 4 N)(NCS). The Th IV  atom is in a ten-coordinate environment of irregular geometry, being bound to the N atoms of the four thio­cyanate ions and to three bidentate nitrate ions. The average Th—N and Th—O bond lengths are 2.481 (10) and 2.57 (3) Å, respectively.

Tris(tetrabutylammonium) tris(nitrato-κ2O,O′)tetrakis(thiocyanato-κN)thorium(IV)

Tris(tetrabutylammonium) tris(nitrato-κ²O,O′)tetrakis(thiocyanato-κN)thorium(IV)