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In the title coordination polymer, [Cu(NCS) 2 (C 12 H 8 N 2 )]  n  , the Cu II  atom is situated on a twofold rotation axis and is coordinated by two N atoms from the bidentate 1,10-phenanthroline ligand and four thio­cyanate groups to confer a CuN 4 S 2  octa­hedral geometry and resulting in a layer structure extending parallel to (100).

acta crystallographica. section e

A second polymorph ofcatena-poly[[(1,10-phenanthroline-κ2N,N′)copper(II)]-di-μ-thiocyanato-κ2N:S;κ2S:N]