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The title compound, [Li 2 (C 9 H 14 N)(C 16 H 36 P 3 )]  n  , is a by-product of the reaction of [Cp(C 5 H 4 CH 2 CH 2 NMe 2 )ZrCl 2 ]  n   with   t  Bu 2 P–P(SiMe 3 )Li in toluene. It is a coordination polymer composed of infinite chains running along [010]. One Li(I) atom is chelated by the cyclo­penta­dienyl ring and and the N atom of the scorpionate ligand and a P atom, whereas the other Li(I) atom is coordinated by the backside of the cyclo­penta­dienyl ring and two P atoms. Both Li(I) atoms adopt a distorted trigonal coordination. The structure was determined from a twinned crystal, but only the data from the main twin component was used. The fraction of components in the crystal was 0.555:0.445 and the twin matrix corresponds to twofold rotation about the  c  axis (    00/0    0/001).

acta crystallographica. section e

catena-Poly[{μ-η5:η5-1-[2-(dimethylamino)ethyl-κN]cyclopentadienyl}-lithium(I)-(μ-1,1,3,3-tetra-tert-butyltriphosphane-κ3P2:P1,P3)lithium(I)]