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In the title compound, [Co(NCS) 2 (C 16 H 16 N 4 O 2 )]  n  , the octa­hedrally coordinated Co II  ion lies on a crystallographic inversion center, with  trans  isothio­cyanate ligands. Pyridyl N-donor atoms and formyl O-donor atoms from exotetra­dentate bis­(4-pyridyl­carbon­yl)piperazine (4-bpfp) ligands link the Co(NCS) 2  units into a [Co(NCS) 2 (4-bpfp)]  n   coordination polymer layer that is oriented parallel to (101). The layers stack along [010] to construct the pseudo-three-dimensional structure.

Poly[[μ4-bis(4-pyridylcarbonyl)piperazine-κ4N:N′:O:O′]bis(thiocyanato-κN)cobalt(II)]

Poly[[μ₄-bis(4-pyridylcarbonyl)piperazine-κ⁴N:N′:O:O′]bis(thiocyanato-κN)cobalt(II)]