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The title compound, [Cu(NCS)(C 12 H 8 N 6 )]  n  , is a self-assembled two-dimensional metal–organic network. The Cu atom is linked by two N atoms from two 3,6-di-4-pyridyl-1,2,4,5-tetra­zine ligands and by the N and S atoms from two thio­cyanate ligands in a distorted tetra­hedral environment. The Cu atom and the thio­cyanate ligand occupy a crystallographic mirror plane  m , and a crystallographic inversion centre is in the middle of the tetra­zine ring, generating the zigzag fashion of the two-dimensional network. The infinite –Cu—SCN—Cu—SCN– chain is due to translational symmetry along the  a  axis. These chains are further connected through the 3,6-di-4-pyridyl-1,2,4,5-tetra­zine ligands that bridge the Cu I  centers, generating a two-dimensional network. There are π—π stacking inter­actions between the pyridine and tetra­zine rings (perpendicular distances of 3.357 and 3.418 Å), with a centroid–centroid distance of 3.6785 (16) Å.

Poly[(μ2-3,6-di-4-pyridyl-1,2,4,5-tetrazine)(μ2-thiocyanato)copper(I)]

Poly[(μ₂-3,6-di-4-pyridyl-1,2,4,5-tetrazine)(μ₂-thiocyanato)copper(I)]