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In the title compound, [Nd(NCS) 3 (C 15 H 15 NO 2 ) 3 ], the Nd III  ion is coordinated by three thio­cyanate anions [Nd—N = 2.489 (8)–2.530 (7) Å] and six O atoms [Nd—O = 2.375 (4)–2.843 (5) Å] from three zwitterionic 2-meth­oxy-6-(4-methyl­phenyl­iminiometh­yl)phenolate ligands in a tricapped trigonal-prismatic geometry. Intra­molecular N—H⋯O hydrogen bonds occur. The crystal packing exhibits weak inter­molecular C—H⋯S hydrogen bonds, π–π inter­actions with a distance of 3.904 (7) Å between the centroids of the aromatic rings, and voids of 101 Å 3 .

Tris[2-methoxy-6-(4-methylphenyliminiomethyl)phenolato-κ2O,O′]tris(thiocyanato-κN)neodymium(III)

Tris[2-methoxy-6-(4-methylphenyliminiomethyl)phenolato-κ²O,O′]tris(thiocyanato-κN)neodymium(III)