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The title compound, [Fe 2 (C 16 H 14 N 2 O 2 ) 2 (NCS) 2 ], is isostructural with the Mn III -containing analogue. Each Fe III  atom is chelated by a tetra­dentate 2,2′-[ethane-1,2-diylbis(nitrilo­methyl­idyne)]diphenolate ligand and by the N atom of a thio­cyanate anion, in a square-pyramidal arrangement. The complex mol­ecules form centrosymmetric dimers, with an Fe—O contact of 2.549 (3) Å,  trans  to each thio­cyanate anion, completing a distorted octa­hedral coordination geometry.

Bis{μ-2,2′-[ethane-1,2-diylbis(nitrilomethylidyne)]diphenolato}bis[(thiocyanato-κN)iron(III)]