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Cyclometallated Pt(II) compounds incorporating the 1,3-di(2-pyridyl)benzene tridentate (N^C^N) pincer ligand have proved highly promising for luminescence applications. 1-3 Such compounds also show significant scope for “tuning” with substitution at various points on the pincer, particularly the central phenyl para to the metal, producing compounds with emissive frequencies across the visible spectrum. 2, 4 Less well-studied, however, is the effect of ligand substitution on the fourth platinum coordination position. It has been shown however, that substitution at this position has significant scope in altering the solid state aggregation of the compounds, and in facilitating intermolecular Pt-Pt interactions. 5

Solvent-induced solid-state structural rearrangement in a novel platinum pincer compound