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approximant [4] and the Hume-Rothery mechanism for the formation of the quasicrystal [5]. For Al-Co-Ni, Ni and Co are located in the most inner and second inner parts, respectively, of the columnar model cluster, indicating the tendency of the close distribution of Ni atoms and the separated distribution of Co atoms. This is consistent with a recent study on the formation of the quasiperiodic Al-Co-Ni surfaces by the scanning tunneling microscopy [6]. The chemical bond and formation of the quasicrystals has been discussed in terms of local clusters around the transition metals. [1] M. Inukai et al., Phil. Mag. 87 (2007) 3003. [2] H. Adachi et al., J. Phys. Soc. Jpn., 45 (1978) 875. [3] K. Hiraga, Adv. Imaging and Electron Phys. 122 (2002) 1. [4] M. Krajči et al., Phys. Rev. B 62 (2000) 243 and ibid. 56 (1997) 3072. [5] A.P. Tsai, Physical Properties of Quasicrystals (Z.M. Stadnik ed., Springer-Verlag, Berlin 2000) p.23. [6] J. Yuhara et al., private communication.

Ni(II) thiosemicarbazone complexes: structural and theoretical investigation