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Sea-salt aerosols are a source of atmospheric bromine responsible for ozone depletion. The availability of bromine from sea-salt aerosols to heterogeneous phase chemical reactions is determined by its local concentration at the aerosol surface. We report here complete surface segregation of bromine in mixed NaCl/NaBr aerosols grown by drying droplets, thus mimicking the atmospheric process by which solid sea-salt aerosols are generated. For d=70  nm solid aerosols, complete surface segregation is observed for solution Br/Cl ratios below 2%. These findings set a size-dependent upper limit on the bromine surface enrichment that can be reached in solid salt aerosols grown from sea-water droplets in the atmosphere

physical review. x

Complete Bromide Surface Segregation in Mixed<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:mi>NaCl</mml:mi><mml:mo>/</mml:mo><mml:mi>NaBr</mml:mi></mml:mrow></mml:math>Aerosols Grown from Droplets

Complete Bromide Surface Segregation in MixedNaCl/NaBrAerosols Grown from Droplets