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We report magnetic properties of a 4f-honeycomb iodide SmI3 made up ofedge-shared network of SmI6 octahedra. High temperature magnetic susceptibilityindicates {\Gamma}7 Kramers doublet ground state of Sm3+ (4f5) ions stabilizedby the spin-orbit coupling and octahedral crystal electric field, whichinteract with Sm-I-Sm bond angle nearly 90 degree. Magnetization measurementsdown to 0.1 K detected antiferromagnetic correlations and an anomaly in themagnetization curve before saturation without a sign of long-range order.Relevance between SmI3 and the antiferromagnetic Kitaev material proposed inthe 4f-electron system is discussed.

SmI3: 4f5 honeycomb magnet with spin-orbital entangled {\Gamma}7 Kramers doublet