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Local configurational disorder can have a dominating role in the formation ofmacroscopic functional responses in strongly correlated materials. Here, we useentropy-stabilization synthesis to create single crystal epitaxial ABO3perovskite thin films with equal atomic concentration of 3d transition metalcations on the B-site sublattice. X-ray diffraction, atomic force microscopy,and scanning transmission electron microscopy ofLa(Cr0.2Mn0.2Fe0.2Co0.2Ni0.2)O3 (L5BO) films demonstrate excellentcrystallinity, smooth film surfaces, and uniform mixing of the 3d transitionmetal cations throughout the B-site sublattice. The magnetic properties arestrongly dependent on substrate-induced lattice anisotropy and suggest thepresence of long-range magnetic order in these exceptionally disorderedmaterials. The ability to populate multiple elements onto a single sublatticein complex crystal structures opens new possibilities to design functionalityin correlated systems and enable novel fundamental studies seeking tounderstand how diverse local bonding environments can work to generatemacroscopic responses, such as those driven by electron-phonon channels andcomplex exchange interaction pathways.

Magnetic anisotropy in single crystal high entropy perovskite oxide La(Cr0.2Mn0.2Fe0.2Co0.2Ni0.2)O3 films