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Scanning tunneling microscopy (STM) and density-functional theory are used to reexamine the structure of the renowned p(4×4)-O/Ag(111) surface oxide. The accepted structural model [C. I. Carlisle et al., Phys. Rev. Lett. 84, 3899 (2000)] is incompatible with the enhanced resolution of the current STM measurements. An "Ag6 model" is proposed that is more stable than its predecessor and accounts for the coexistence of the p(4×4) and a novel c(3×5sqrt(3))rect phase. This coexistence is an indication of the dynamic complexity of the system that until now has not been appreciated

physical review letters

Revisiting the Structure of the<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi>p</mml:mi><mml:mo stretchy="false">(</mml:mo><mml:mn>4</mml:mn><mml:mo>×</mml:mo><mml:mn>4</mml:mn><mml:mo stretchy="false">)</mml:mo></mml:math>Surface Oxide on Ag(111)

Revisiting the Structure of thep(4×4)Surface Oxide on Ag(111)