English (United Kingdom)

https://curated-unify.zendy.io/wp-json/zendy-region/v1/featured_content/oa?rat=en

https://curated-unify.zendy.io/wp-json/zendy-region/v1/highlighted_journal/

Global: Zendy Plus annual

Presents the access of premium content as premium feature

Premium Content

Presents the keyphrase highlighting as premium feature

Keyphrase Highlighting

Presents the summarisation as premium feature

Summarisation

Insights

Presents the pdf analysis as premium feature

PDF Analysis

Presents the zaia usage as premium feature

ZAIA

Global: Zendy Plus monthly

Global: Zendy Tools annual

Global: Zendy Tools monthly

Global: Zendy Free Plan

The underlying mechanism for Adaptive Feedback Control in the experimentalphotoisomerization of NK88 in methanol is exposed theoretically. With givenlaboratory limitations on laser output, the complicated electric fields areshown to achieve their targets in qualitatively simple ways. Further, controlover the cis population without laser limitations reveals an incoherentpump-dump scenario as the optimal isomerization strategy. In neither case arethere substantial contributions from quantum multiple-path interference or fromnuclear wavepacket coherence. Environmentally induced decoherence is shown tojustify the use of a simplified theoretical model.Comment: 10 pages, 3 figures, to be published in Phys. Rev. Let

Mechanisms in Adaptive Feedback Control: Photoisomerization in a Liquid