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The interplay between inter- and intra-chain charge transport in bulkpolythiophene in the hopping regime has been clarified by studying theconductivity as a function of frequency (up to 3 THz), temperature and dopinglevel. We present a model which quantitatively explains the observed crossoverfrom quasi-one-dimensional transport to three-dimensional hopping conductionwith increasing doping level. At high frequencies the conductivity is dominatedby charge transport on one-dimensional conducting chains.

Dopant-Induced Crossover from 1D to 3D Charge Transport in Conjugated Polymers