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Using an electronic tight-binding theory we calculate the nonlinearmagneto-optical response from an x-Cu/1Fe/Cu(001) film as a function offrequency and Cu overlayer thickness (x=3 ... 25). We find very strongspin-polarized quantum well oscillations in the nonlinear magneto-optical Kerreffect (NOLIMOKE). These are enhanced by the large density of Fe $d$ statesclose to the Fermi level acting as intermediate states for frequency doubling.In good agreement with experiment we find two oscillation periods of 6-7 and 11monolayers the latter being more pronounced.Comment: 12 pages, Revtex, 3 postscript figure

Theory for Spin-Polarized Oscillations in Nonlinear Optics due to Quantum Well States