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Control over the product branching ratio in the photodissociation of Na 2 intoNa(3s)+ Na(3p) , and Na(3s)+ Na(3d) is demonstrated using a two-photonincoherent interference control scenario. Ordinary pulsed nanosecond lasersare used and the Na 2 is at thermal equilibrium in a heat pipe. Results showa depletion in the Na(3d) product of at least 25% and a concomitant increasein the Na(3p) yield as the relative frequency of the two lasers is scanned.1We report the experimental...

physical review letters

Experimental Observation of Laser Control: Electronic Branching in the Photodissociation of N<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">a</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>

Experimental Observation of Laser Control: Electronic Branching in the Photodissociation of Na2