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High-quality polarized-emission cross sections for the )..cap alpha..)/sub 5/ = chemically bondJ = 1,M/sub J/>..-->..)..cap alpha..)/sub 7/ and )..cap alpha..)/sub 5/..-->..)..cap alpha..)/sub 4/ transitions in the )..cap alpha..) = )(2p)/sup 5/(3p)) multiplet (lifetime 20 ns) have been measured in a crossed-beam experiment. For the )..cap alpha..)/sub 5/..-->..)..cap alpha..)/sub 7/ transition we observe a strong preference for the chemically bondM/sub J/chemically bond = 0 orientation. The small cross section for the chemically bondM/sub J/chemically bond = 1 orientation can be understood qualitatively from the model potentials of Hennecart and Masnou-Seeuws by the strong coupling to the )..cap alpha..)/sub 4/ and )..cap alpha..)/sub 6/ states (avoided crossings), which is absent for the ..cap omega.. = chemically bondM/sub J/chemically bond = 0/sup -/ molecular potentials because of the constraint of reflection symmetry.

physical review letters

Polarization Effects in Collision-Induced Intramultiplet Mixing for<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msup><mml:mrow><mml:mi mathvariant="normal">Ne</mml:mi></mml:mrow><mml:mrow><mml:mo>*</mml:mo><mml:mo>*</mml:mo></mml:mrow></mml:msup></mml:mrow><mml:mo>{</mml:mo><mml:mrow><mml:msup><mml:mrow><mml:mn /><mml:mo>(</mml:mo><mml:mn>2</mml:mn><mml:mi>p</mml:mi><mml:mo>)</mml:mo><mml:mn /></mml:mrow><mml:mrow><mml:mn>5</mml:mn></mml:mrow></mml:…

Polarization Effects in Collision-Induced Intramultiplet Mixing forNe**{(2p)5