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Hybrid matter-photon entanglement is the building block for quantum networks.It is very favorable if the entanglement can be prepared with a highprobability. In this paper, we report the deterministic creation ofentanglement between an atomic ensemble and a single photon by harnessingRydberg blockade. We design a scheme that creates entanglement between a singlephoton's temporal modes and the Rydberg levels that host a collectiveexcitation, using a process of cyclical retrieving and patching. The hybridentanglement is tested via retrieving the atomic excitation as a second photonand performing correlation measurements, which suggest an entanglement fidelityof 87.8%. Our source of matter-photon entanglement will enable the entanglingof remote quantum memories with much higher efficiency.

Deterministic Time-Bin Entanglement between a Single Photon and an Atomic Ensemble