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Above-bandgap optical illumination induces a transformation from tiltedtetragonal-like (T-like) and rhombohedral-like (R-like) phases to an untiltedT-like phase in compressively strained BiFeO3. Optical excitation leads to anout-of-plane lattice expansion in the T-like phase. The transformation proceedsin regions with boundaries between the T-like and tilted R-like and tiltedT-like phases, consistent with the motion of a boundary. The optically inducedtransformation indicates that there are new optically driven routes towardsnanosecond-scale control of phase transformations in ferroelectrics andmultiferroics.

Nanosecond Optically Induced Phase Transformation in Compressively Strained BiFeO3 on LaAlO3