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Magnetic structures of organic Mott insulators X[Pd(dmit)2]2 (X=Me4P, Me4Sb),of which electronic states are located near quantum spin liquid (X=EtMe3Sb),are demonstrated by 13C NMR. Antiferromagnetic spectra and nuclear relaxationsshow two distinct magnetic moments within each Pd(dmit)2 molecule, which cannotbe described by single band dimer-Mott model and requires intramolecularelectronic correlation. This unconventional fragmentation of S = 1/2 electronspin with strong quantum fluctuation is presumably caused by nearly degeneratedintramolecular multiple orbitals, and shares a notion of quantum liquids whereelectronic excitations are fractionalized and S = 1/2 spin is no longer anelementary particle.

Fragmented Electronic Spins with Quantum Fluctuations in Organic Mott Insulators near Quantum Spin Liquid