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Metal deposition on oxide surfaces usually results in adatoms, clusters, orislands of the deposited material, where defects in the surface often act asnucleation centers. Here an alternate configuration is reported. After thevapor deposition of Fe on the In$_2$O$_3$(111) surface at room temperature,ordered adatoms are observed with scanning tunneling microscopy. These areidentical to the In adatoms that form when the sample is reduced by heating inultrahigh vacuum. Density functional theory (DFT) calculations confirm that Feinterchanges with In in the topmost layer, pushing the excess In atoms to thesurface where they arrange as a well-ordered adatom array.

Well-Ordered In Adatoms at the In$_2$O$_3$(111) Surface Created by Fe Deposition